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Concurrent magnetic and structural reconstructions at the interface of (111)-oriented L a0.7 S r0.3Mn O3/LaFe O3

Abstract

We observe an induced switchable magnetic moment of
1.6
±
0.40
μ
B
/
Fe
for the nominally antiferromagnetic
LaFe
O
3
extending two to four interface layers into the non–charge transfer system
L
a
0.7
S
r
0.3
Mn
O
3
/
LaFe
O
3
/
SrTi
O
3
(
111
)
. Simultaneously a mismatch of oxygen octahedra rotations at the interface implies an atomic reconstruction of reduced symmetry at the interface, reaching two to five layers into
LaFe
O
3
. Density functional theory of a structure with atomic reconstruction and different correlation strength shows a ferrimagnetic state with a net Fe moment at the interface. Together these results suggest that engineered oxygen octahedra rotations, affecting the local symmetry, affect electron correlations and can be used to promote magnetic properties.

Category

Academic article

Client

  • Sigma2 / NN9301K
  • Research Council of Norway (RCN) / 231290

Language

English

Author(s)

  • Ingrid Hallsteinsen
  • Magnus Moreau
  • A Grutter
  • Martin Nord
  • Per Erik Vullum
  • DA Gilbert
  • Torstein Bolstad
  • Jostein Grepstad
  • Randi Holmestad
  • Sverre Magnus Selbach
  • AT N'Diaye
  • BJ Kirby
  • E Arenholz
  • Per Thomas Martin Tybell

Affiliation

  • Norwegian University of Science and Technology
  • Lawrence Berkeley National Laboratory
  • USA
  • SINTEF Industry / Materials and Nanotechnology

Year

2016

Published in

Physical Review B. Condensed Matter and Materials Physics

ISSN

1098-0121

Volume

94

Issue

20

Page(s)

201115-1 - 201115-6

View this publication at Cristin